职称：教授，博士生导师

教育部新世纪优秀人才

专业：物理化学

Email：shengbin.lei@tju.edu.cn

招生情况：每年招收博士生1-2人，硕士生2人。

ResearchID个人主页：http://www.researcherid.com/rid/D-9089-2011

1.教育经历

1999/9-2002/7：中科院化学研究所，博士，物理化学，导师：王琛研究员

1996/9-1999/7：山东大学化学系，硕士，物理化学，导师：陈慎豪教授

1992/9-1996/7：山东大学化学系，本科

2.研究工作经历

2015/8至今：天津大学，天津市分子光电科学重点实验室，博士生导师

2009/9-2015/7：哈尔滨工业大学，微系统与微结构制造教育部重点实验室，博士生导师

2006/7-2009/8:比利时鲁汶天主教大学化学系，光化学与光谱实验室，博士后

2005/1-2006/7:中国科学院化学研究所分子纳米结构与纳米技术院重点实验室，副研究员

2002/7-2004/12:中国科学院化学研究所分子纳米结构与纳米技术院重点实验室，助理研究员

3. 个人简介

主要从事有机二维材料与器件、表面物理化学研究。近年二维聚合物的形成机制和物理化学性质、表面限域的动态共价化学研究方面取得了一系列科研成果。提出了二维超分子网格的浓度控制和模板分子诱导策略，并成功将之应用于表面动态化学反应的调控，揭示了表面动态化学反应中的关键控制因素，初步实现了对动态共价反应从体相到界面的控制；发展了一种操作简便、条件温和的二维聚合物表面合成方法，实现了大范围、连续、具有规整结构的系列二维聚合物的室温制备；实验结合理论计算研究了二维聚合物及其与石墨烯复合物的化学与能带结构，探索了其在电化学储能及光电传感方面的应用。

在Angew. Chem. Int. Ed., J. Am. Chem. Soc.,Nano Lett.,Adv. Mater.,ACSNano,Nanoscale,Chem. Comm.,Chem. Eur. J.等杂志发表SCI收录论文120余篇，为Top. Curr. Chem., Chem. Soc. Rev., Angew. Chem. Int. Ed., Nanoscale, Chem. Comm., CrystEngComm撰写综述六篇。

论文被引用4200余次，其中近五年来被引用2000余次。其中10篇论文单篇引用超过100次，第一作者论文单篇最高引用次数超过次。个人H因子34(http://www.researcherid.com/rid/D-9089-2011)。获2005年度中国化学会青年化学奖，2009年获教育部新世纪优秀人才计划支持。J. Am. Chem. Soc.,Nanoscale, Chem. Eur. J., Chem. Comm., Langmuir, Polymer, Soft Matter, ChemPhysChem, Sci. China Chem.等杂志审稿人，比利时弗拉芒区基金(the research foundation Flanders)评阅人。《Transactions of Tianjin University》（即《天津大学学报（英文版）》）编委

4.主要研究方向

1)有机二维材料与器件

致力于发展具有光电功能的有机二维材料，尤其是薄膜材料的制备技术，探索其在场效应晶体管、记忆存储器件、光检测器等领域的应用。

2) 表面限域的动态共价化学

在动态共价化学反应中表面限域作用不仅体现在对产物的选择和放大作用，而且在二维聚合物的生长过程中范德华外延作用还可以诱导生成更加长程有序的结构。本研究方向主要致力于探索表面限域作用对动态共价体系的产物选择和反应过程的新奇效应以及利用表面限域效应制备长程有序的二维聚合物材料。

5.主持或参加科研项目及人才基金项目情况

1. 国家自然科学基金委面上项目，21572157，席夫碱二维聚合物的表面反应制备及性质研究，2016.1－2019.12，65万，正在进行中，主持。

2. 国家自然科学基金委面上项目，21373070，石墨烯－有机半导体界面结构及结构与性能关系，2014.1－2017.12，82万，已结题，主持。

3. 国家自然科学基金委面上项目，21173061，固液界面多孔分子网格的功能化， 2012.1－2015.12，61万，已结题，主持。

4. 教育部新世纪优秀人才，2010.1-2012.12，50万，已结题，主持。

5. 教育部留学归国人员科研启动基金, 2013.1-2015.12,3.0万, 已结题，主持。

6. 校985领军学者与团队，2011.1-2012.12，32万，已结题，主持。

7. 校基础研究杰出人才培育计划，2011.1-2012.12，18万，已结题，主持。

8. 新型TiO₂/石墨烯复合材料的制备及其催化机理研究，水资源与水环境国家重点实验室开放课题，2011.7-2014.6，10万，已结题，主持。

9. 国家自然科学基金委面上项目，50573089，导电高分子薄膜的结构与性能研究，2006.1－2008.12，26万，已结题，主持。

10. 国家自然科学基金委面上项目（青年），20303023，多组分表面分子纳米结构构筑与表征，2004.1－2006.12，24万，已结题，主持。

11. 国家纳米中心协作实验室课题，蛋白质生物纳米传感器的研究，2004.7-2006.6， 50万，已结题，参加。

12. 中科院知识创新工程重大项目，2002CCA0310，《若干纳米器件的基础性研究》子课题：纳米结构的检测与表征，2001.1-2005.12，100万，已结题，参加。

13. 基金委面上项目，20073053，有机分子的可控吸附与组装的扫描探针显微研究，2001.1－2003.12，25万，已结题，参加。

14. 科技部973项目，G2000077501，973《创造新物质的分子工程学研究》子课题：单分子和纳米基元的结构研究，2000.9-2005.9，133万，已结题，参加。

6.获奖

获2005年中国化学会青年化学奖

2009年获教育部新世纪优秀人才计划支持

7.近五年论文

2018

1. Chunhua Liu, Eunsol Park, Jie Liu, Yanxia Yu, Yinghua Jin, Wei Zhang*, Shengbin Lei*, Wenping Hu, Surface-Confined Dynamic Covalent System Driven by Olefin Metathesis

Angew. Chem. Int. Ed. 2018,57(7), 1869-1873.

2. Chunhua Liu,Eunsol Park, Jie Liu, Yanxia Yu, Yinghua Jin, Wei Zhang*, Shengbin Lei*, Wenping Hu, Effective Separation of Arylenevinylene Macrocycles with a Surface Confined Two-Dimensional Imine Covalent Organic Framework,

Angew. Chem. Int. Ed.2018,DOI: 10.1002/anie.201803937.

3. Chunhua Liu, Ling Yang, Yan Wang, Shengbin Lei*,Substrate effects in the supramolecular assembly of 2,4,6-tris(4-bromophenyl)-1,3,5-triazine on graphite and graphene

J. Phys. Chem. C, 2018,10.1021/acs.jpcc.8b02979.

4. Jiang Sun, Shengbin Lei, Guest-Induced Structural Transformation and Its Effect on the Redistribution of the Surface Confined Combinatorial Libraries

J. Phys. Chem. C, 2018, 10.1021/acs.jpcc.8b03215.

5. Yanxia Yu, Nerea Bilbao, Lander Verstraete, Shengbin Lei*, and Steven De Feyter,* The impact of grafted surface defects on the on-surface Schiff-base chemistry at the solid-liquid interface

Chem. Commun. 2018,Submitted.

6. Zongxia Guo,* Ping Yu, Kai Sun, Shengbin Lei, Yuanping Yi and Zhibo Li*, Role of halogenhalogen interactions in the 2D crystallization of n-semiconductors at the liquid–solid interface

Phys. Chem. Chem. Phys., 2018, 19(47), 31540-31544.

7. Yumin Chen, Ke Deng*, Shengbin Lei, Rong Yang, Tong Li, Yuantong Gu, Yanlian Yang*, Xiaohui Qiu*, Chen Wang, Single-molecule Insights into Surface-mediated Homochirality in Hierarchical Peptide Assembly

Nature Comm., 2018, accepted.

2017

8. Yanxia Yu, Chunhua Liu, Jiang Sun, Shengbin Lei*, DynamicCovalentChemistry ofImine Polymers at Liquid/solid Interfaces Investigated by Scanning Tunneling Microscopy

RSC Advances, 2017,7, 11496 - 11502.

9. Jiang Sun,Yanxia Yu, Chunhua Liu, Shengbin Lei*,Surface- and Guest-Promoted Product Selection from a Dynamic Covalent Library: A Scanning Tunneling Microscopic Study

J. Phys. Chem. C, 2017,121, 3437-3444.

10. Yanxia Yu, Ya li Zheng,Shengbin Lei*, From a Two-Dimensional Supramolecular Network to One-Dimensional Covalent Polymer at the Liquid/Solid Interface: Insight into the Role of the Stoichiometric Ratio of the Precursors

J. Phys. Chem. C, 2017,121 (1), 593-599.

2016

11. Chunhua Liu, Wei Zhang, Qingdao Zeng, Shengbin Lei*,A PhotoresponsiveTwo-Dimensional CovalentOrganicFramework: Surface-Confined Synthesis, Isomerization and Controlled Guest Capture and Release

Chem. Eur. J. 2016,22, 6768-6773.

12. Lirong Xu, Yanxia Yu, Jianbin Lin, Xin Zhou,* Wei Quan Tian,Damian Nieckarz, Pawel Szabelski,*Shengbin Lei,*On-Surface Synthesis of Two-dimensional Imine Polymers with Tunable Band Gap: a Combined STM, DFT and Monte Carlo Investigation

Nanoscale,2016,8, 8568 - 8574.

13. Yanxia Yu, Jianbin Lin, Yan Wang, Qingdao Zeng, Shengbin Lei,* Room Temperature On-Surface Synthesis of Crystalline Two-Dimensional Imine Polymers at the Solid/Liquid Interface: Concentration Takes Control

Chem. Comm.,2016,52, 6609-6612.

14. Jiang Sun, Xin Zhou* and Shengbin Lei*, Host-Guest Architectures with a Surface Confined Imine Covalent Organic Framework as Two-Dimensional Host Networks

Chem. Comm., 2016,52, 8691-8694.

15. Yanxia Yu, Ling Yang,*Chunhua Liu, Wei-Quan Tian,Yan Wang,* Shengbin Lei*, Hierarchical Construction of Cross-Junction of Molecular Wires with Covalent and Noncovalent Interactions at the Liquid/Solid Interface

Chem. Comm., 2016, 52, 8317-8320.

16. Chunhua Liu, Yanxia Yu,Wei Zhang, Qingdao Zeng,Shengbin Lei*,Room Temperature Synthesis of Covalent Organic Frameworkswith Boronic Ester Linkage at the Liquid/Solid interface

Chem. Eur. J, 2016,22, 18412-18418.

17. Jia Zhang, Chao Zhao, Na Liu, Huanxi Zhang, Jingjing Liu, Yong Qing Fu, Bin Guo, Zhenlong Wang*, Shengbin Lei, PingAn Hu*, Tunable electronic properties of graphene through controlling bonding configurations of doped nitrogen atoms

Scientific Reports, 2016,6, 28330.

2015

18. Lirong Xu, Lili Cao, Zongxia Guo, Zeqi Zha,Shengbin Lei*,Side-Functionalized Two-Dimensional Polymers Synthesized via On-Surface Schiff-Base Coupling

Chem. Comm.,2015,51, 8664 - 8667.

19. Xiu-Ling Sun, Li-Xia Fan, Yong-Jing Yang, Zongxia Guo*, Wei Quan Tian, Shengbin Lei*,Synthesis of One Dimensional Schiff Base Polymers Containing Oligothiophene Building Block on the Graphite Surface

Chem. -Eur J., 2015, 21, 6898-6905.

20. Xiuling Sun, Lixia Fan, Xin Zhou*, Wei Quan Tian, Zongxia Guo*, Zhibo Li,Xiaokang Li,Shengbin Lei*, SurfaceConfinedSynthesis of Porphyrin ContainingTwo-Dimensional Polymers: the Effect of Rigidity and Preferential Adsorption of Building Blocks

Chem. Comm., 2015,51, 5864-5867.

21. Xin Zhou, Longtao Jiang, Shengbin Lei*, Wei Quan Tian*, Gaohui Wu*,Micro-mechanism in Self-lubrication of TiB₂/Al Composite

ACS Appl. Mater. Interfaces, 2015, 7, 12688−12694.

22. Zeqi Zha, Lirong Xu, Zhikui Wang, Qinmin Pan,Shengbin Lei*, 3D Graphene Functionalized by Covalent Organic Framework Thin Film as Capacitive Electrode in Alkaline Media

ACS Appl. Mater. Interfaces, 2015,7 (32), pp 17837–17843.

23. Yanxia Yu, Jiang Sun, Shengbin Lei*,Surface Confined Synthesis of One-DimensionalSchiff Base PolymersInvestigated byScanning Tunneling Microscopy

J. Phys. Chem. C, 2015, 119,16777–16784.

24. Yanqiu Jiang, Zongxia Guo, Shengbin Lei*,The Assembling of Poly (3-Octyl-Thiophene) on CVD Grown Single Layer Graphene

Scientific Reports, 2015,5, 17720; doi: 10.1038/srep17720.

25. Junyan Zhu, Zeyuan Dong*, Shengbin Lei, Lili Cao, Bing Yang, Wenfang Li, Yuanchao Zhang, Junqiu Liu*, and Jiacong Shen,Design of Aromatic Helical Polymers for STM Visualization : Imaging of Single and Double Helices with a Pattern of p –p Stacking

Angew. Chem. Int. Ed.,2015, 54(10), 3097-3101.

2014

26. Lirong Xu, Xin Zhou, Wei Quan Tian, Teng Gao, Yan Feng Zhang, Shengbin Lei,* and Zhong Fan Liu,Surface Confined Single Layer Covalent Organic Framework on Single Layer Graphene Grown on Copper Foil

Angew. Chem. Int. Ed.,2014, 53(36), 9564-9568.

27. Xiuling Sun, Youbing Mu, Jia Zhang, Xiaona Wang, Pingan Hu, Xiaobo Wan,* Zongxia Guo,* and Shengbin Lei*,Tuning Self-Assembly of Oligothiophenes on CVD Graphene: Effect of Functional Group, Solvent and Substrate

Chem. -Asian J., 2014, 9(7), 1888-1894.

28. Lili Cao, Lirong Xu, Dahui Zhao, Kazukuni Tahara, Yoshito Tobe, Steven De Feyter, Shengbin Lei*, Efficient Molecular Recognition Based on Nonspecific van der Waals Interaction at the Solid/Liquid Interface

Chem. Commun.2014, 50 (80), 11946-11949.

29. Min Li, Peng Xie, Ke Deng, Yan-Lian Yang, Sheng-Bin Lei, Zhong-Qing Wei,* Qing-Dao Zeng* and Chen Wang*, A dynamic study of the structural change in thebinary network in response to guest inclusion

Phys. Chem. Chem. Phys., 2014, 16, 8778-8782.

30. Kazukuni Tahara, Jinne Adisoejoso, Koji Inukai, Shengbin Lei, Aya Noguchi, Bing Li, Willem Vanderlinden, Steven De Feyter* and Yoshito Tobe*,Harnessing by a diacetylene unit: a molecular design for porous two-dimensional network formation at the liquid/solid interface

Chem. Commun.2014, 50,2831-2833.

31. Li Wang, Xingping Lu, Shengbin Lei and Yonghai Song*, Graphene-based polyaniline nanocomposites: preparation, properties and applications

J. Mater. Chem. A, 2014, 2, 4491-4509.

32. Liming Qin, Jie Zhao, Shengbin Lei, and Qinmin Pan*, A Smart “Strider” Can Float on Both Water and Oils,

ACS Appl. Mater. Interfaces, 2014, 6, 21355-2136.

2013

33. Lirong Xu, Xin Zhou, Yanxia Yu, Wei Quan Tian*, Jun Ma,Shengbin Lei*, Surface Confined Crystalline Two-Dimensional Covalent Organic Frameworksvia on Surface Schiff-Base Coupling

ACS nano, 2013, 9, 8066-8073.

34. Xiuling Sun, Jia Zhang, Xiaona Wang, Cuiyun Zhang, Pingan Hu,Youbing Mu, Xiaobo Wan, Zongxia Guo* andShengbin Lei*,“Oligothiophenes on CVDGrapheneGrown onMulti-crystallineCopperFoil: SupramolecularAssembling and Morphology Impact”

Chem. Commun.2013, 49, 10317-10319.

35. Lirong Xu, Liu Yang, Lili Cao, Tian Li, Shusen Chen, Dahui Zhao*,Shengbin Lei*, Jun Ma, “Effect of Bulky Substituent on the Self-Assembly and Mixing Behavior of Arylene Ethynylene Macrocycles at the Solid/Liquid Interface”

Phys. Chem. Chem. Phys., 2013, 15, 11748-11757.

36. Yong-Tao Shen, Ning-Bo Zhu, Xue-Mei Zhang,Shengbin Lei, Zhongqing Wei, Min Li,* Dahui Zhao,* Qing-Dao Zeng,* Chen Wang*，“Assemblies at the Liquid-Solid Interface: Chirality Expression from Molecular Conformers”

ChemPhysChem, 2013, 14, 92–95.

37. Xiaona Wang, Xiuling Sun, Ping An Hu,* Jia Zhang, Lifeng Wang, Wei Feng, Shengbin Lei, Bin Yang, and Wenwu Cao, Colorimetric Sensor Based on Self-Assembled Polydiacetylene/Graphene-Stacked Composite Film for Vapor-Phase Volatile Organic Compounds

Adv. Funct. Mater., 2013, 23, 6044-6050.